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Current Gallery is a neat place to see and perhaps purchase some local artists' work, but its best reputation (among locals) is as a DIY indie music venue by night. Check local listings and their website to find out what's going on.
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An excellent free library with a one-of-a-kind archive of rare books and documents, including many related to Edgar Allan Poe and H.L. Mencken, and an extensive 16mm film collection including many avant garde rarities. The children's department has a goldfish pond.
Basilica of the Assumption
A small house museum of America's first native-born saint, beatified by the Vatican for her relief work and founding of Catholic schools, and for three miraculous cures performed towards the end of her life.
This is a beautiful 1914, former vaudeville and early movie theater. It is the biggest performing arts venue downtown, and hosts frequent Broadway productions.
This early 19th century church is a most atmospheric and tortuous place of famous Baltimore residents including, most famously, Edgar Allan Poe, as well as James McHenry (signer of the U.S. Constitution), Samuel Smith, former city mayors, and others. Halloween is the city's favorite time to visit, but any midnight dreary would be most appropriate (although this would involve an attempt of questionable legality to slip past the gates). It is custom to leave a penny behind his grave marker, which in turn pays for its upkeep! There are tours, but they are subect to availability April–November: F 6:30PM, Sa 10AM, minimum fifteen people, with reservations required, $5. Private tours are always an option, but must be set up at least two weeks in advance, and fees will vary.
Baltimore Arena or Royal Farms Arena
Baltimore city's largest indoor venue is host to frequent sporting and other major performances. It's an old clunker, and they're looking to replace it, but it's still fine to bring your family here.